Bob Marley and The Wailers

Despite the breakup, Marley continued recording as "Bob Marley & The Wailers". His new backing band included brothers Carlton and Aston "Family Man" Barrett on drums and bass respectively, Junior Marvin and Al Anderson on lead guitar, Tyrone Downie and Earl "Wya" Lindo on keyboards, and Alvin "Seeco" Patterson on percussion. The "I Threes", consisting of Judy Mowatt, Marcia Griffiths, and Marley's wife, Rita, provided backing vocals.

In 1975, Marley had his international breakthrough with his first hit outside Jamaica, "No Woman, No Cry," from the Natty Dread album. This was followed by his breakthrough album in the US, Rastaman Vibration (1976), which spent four weeks on the Billboard charts Top Ten.

In December 1976, two days before "Smile Jamaica", a free concert organized by the Jamaican Prime Minister Michael Manley in an attempt to ease tension between two warring political groups, Marley, his wife, and manager Don Taylor were wounded in an assault by unknown gunmen inside Marley's home. Taylor and Marley's wife sustained serious injuries, but later made full recoveries. Bob Marley received minor wounds in the chest and arm. The shooting was thought to have been politically motivated, as many felt the concert was really a support rally for Manley. Nonetheless, the concert proceeded, and an injured Marley performed as scheduled, two days after the attempt. When asked why, Marley responded, "the people who are trying to make this world worse aren’t taking a day off. How can I?".^{[citation needed]} The members of the group Zap Pow – which had no radical religious or political beliefs – played as Bob Marley's backup band before a festival crowd of 80,000 while members of the Wailers were still missing or in hiding.^[19]

Marley left Jamaica at the end of 1976 for England, where he recorded his Exodus and Kaya albums. Exodus stayed on the British album charts for 56 consecutive weeks. It included four UK hit singles: "Exodus", "Waiting In Vain", "Jamming", "One Love", and a rendition of Curtis Mayfield's hit, "People Get Ready". It was here that he was arrested and received a conviction for possession of a small quantity of cannabis while traveling in London.

In 1978, Marley performed at another political concert in Jamaica, the One Love Peace Concert, again in an effort to calm warring parties. Near the end of the performance, by Marley's request, Manley and his political rival, Edward Seaga, joined each other on stage and shook hands.

Babylon by Bus, a double live album with 13 tracks, was released in 1978 to critical acclaim. This album, and specifically the final track "Jammin'" with the audience in a frenzy, captured the intensity of Marley's live performances.

Survival, a defiant and politically charged album, was released in 1979. Tracks such as "Zimbabwe", "Africa Unite", "Wake Up and Live", and "Survival" reflected Marley's support for the struggles of Africans. His appearance at the Amandla Festival in Boston in July 1979 showed his strong opposition to South African apartheid, which he already had shown in his song "War" in 1976. In early 1980, he was invited to perform at the April 17 celebration of Zimbabwe's Independence Day.

Uprising (1980) was Bob Marley's final studio album, and is one of his most religious productions, including "Redemption Song" and "Forever Loving Jah". It was in "Redemption Song" that Marley sang the famous lyric,

Confrontation, released posthumously in 1983, contained unreleased material recorded during Marley's lifetime, including the hit "Buffalo Soldier" and new mixes of singles previously only available in Jamaica.